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By B R Coles

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It appeared to us that the abrupt change in intramolecular dimensions of the cationic complexes is a most crucial point in the cooperative spin transition process in a solid, because it obviously induces changes in lattice vibrations and elastic properties, which initiate further spin state changes. This is the background which stimulated us to develop the "Elastic Interaction and Lattice Expansion (EILE)" model to describe quantitatively the cooperative spin transition in solids. 38 ,54 It is, thereby, of fundamental interest to know what the individual contributions to the total change of 43 2500 o > 100 Fig.

Lalor, J. Chern. Soc. (Dalton), (1973): 718. J. Ens1ing, P. Gut1ich, and L. Rosch, Z. Naturforsch, 30b: 850 (1975) • H. Mosbaek, Acta. Chern. A, 29:957 (1975). B. A. Sosinsky, N. Nor ern , and R. G. Shong, Inorg. , 21: 4229 (1982). M. E1ian and R. Hoffmann,Inorg. , 14:1058 (1975). R. H. Herber, W. R. Kingston, and G. K. Wertheim, Inorg. , 2:153 (1963). P. W. Jones, Can. J. , 51:405 (1973). R. Robinette and R. L. Collins, J. Chern. , 57:4319 (1972). G. M. Bancroft and E. T. Libbey, J, Chern. Soc.

A), (1970): 956. 25 SPIN TRANSITION IN IRON COMPOUNDS Philipp Gutlich Institut fur Anorganische und Analytische Chemie Johannes-Gutenberg-Universitat 0-6500 Mainz, West Germany 1. INTRODUCTION First-row transition metal complexes with d 4 up to d 7 electron configuration in octahedral ligand fields (and dB electron configuration in six-coordinate complexes of lower symmetry) may undergo temperature dependent high spin (BS) ~ low spin (LS) transition, provided the ligand field strength (~), including low symmetry contributions,becomes comparable in magnitude with the mean spin pairing energy (P).

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